Abstract. Nitrogen-doped graphene sheets (NGS) were obtained using a simple hydrothermal reaction with graphene oxide and hexamethylenetetramine (HMT). HMT plays important roles in both reducing graphene oxide and doping nitrogen into the graphene sheets. The prepared nitrogen-doped graphene sheets reduced by hexamethylenetetramine (NGS-HMT) have a high nitrogen (8.62 atom%) content, in wh…